| Schauspieler | Rolle | Synchronsprecher | ||
| Will Smith Will Smith | Agent Jay / James Darrell Edwards III | Jan Odle Jan Odle | ||
| Tommy Lee Jones Tommy Lee Jones | Agent Kay / Kevin Brown | Ronald Nitschke Ronald Nitschke | ||
| Joel Brady | 1969 Man in Elevator | Jeffrey Wipprecht Jeffrey Wipprecht | ||
| Jack O'Connell II | 1969 MIB HQ Guard | Klaus Lochthove Klaus Lochthove | ||
| James Martin Kelly | 1969 NYPD Cop #1 | Kaspar Eichel Kaspar Eichel | ||
| Will McLaughlin | 1969 NYPD Cop #2 | Frank Ciazynski | ||
| Will Arnett Will Arnett | Agent AA (Partner von J, 1969) | Sven Hasper | ||
| Woodie King Jr. | 2012 MIB HQ Guard | Klaus Lochthove Klaus Lochthove | ||
| Emma Thompson Emma Thompson | Agent Oh | Monica Bielenstein Monica Bielenstein | ||
| Josh Brolin Josh Brolin | Agent Kay / Kevin Brown (jung) | Florian Halm Florian Halm | ||
| Alice Eve | Agent Oh (jung) | Maria Koschny Maria Koschny | ||
| Victor Joel Ortiz | Air Force MP #1 | Tino Kießling Tino Kießling | ||
| Charlie Barnett | Air Force MP #2 | Jeffrey Wipprecht Jeffrey Wipprecht | ||
| David Rasche | Agent X | Hans-Jürgen Dittberner Hans-Jürgen Dittberner | ||
| Bill Hader Bill Hader | Andy Warhol | Peter Flechtner Peter Flechtner | ||
| Jemaine Clement Jemaine Clement | Boris, die Bestie | Torsten Michaelis Torsten Michaelis | ||
| Jared Christopherson | Apollo 11 Reporter | Bodo Wolf Bodo Wolf | ||
| Lenny Venito | Bowlingkugel-Kopf | Michael Pan Michael Pan | ||
| Anthony J. Gallo | Four-Armed Alien | Klaus Lochthove Klaus Lochthove | ||
| Mike Colter | Colonel Edwards | Oliver Siebeck Oliver Siebeck | ||
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