| Schauspieler | Rolle | Synchronsprecher | ||
| Sir John Hurt Sir John Hurt | Control | Jürgen Thormann Jürgen Thormann | ||
| Gary Oldman Gary Oldman | George Smiley | Udo Schenk | ||
| Benedict Cumberbatch Benedict Cumberbatch | Peter Guillam | Tommy Morgenstern Tommy Morgenstern | ||
| Colin Firth Colin Firth | Bill Haydon | Tom Vogt Tom Vogt | ||
| Mark Strong Mark Strong | Jim Prideaux | Oliver Siebeck Oliver Siebeck | ||
| Tom Hardy Tom Hardy | Ricki Tarr | Daniel Fehlow Daniel Fehlow | ||
| Ciarán Hinds | Roy Bland | Bernd Rumpf Bernd Rumpf | ||
| David Dencik | Toby Esterhase | Andreas Petri | ||
| Toby Jones Toby Jones | Percy Alleline | Lutz Schnell Lutz Schnell | ||
| Simon McBurney | Oliver Lacon | Cusch Jung | ||
| Stephen Graham Stephen Graham | Jerry Westerby | Uwe Büschken Uwe Büschken | ||
| Stuart Graham | Pfarrer | Frank Röth Frank Röth | ||
| Nick Hopper | Alwyn | Andreas Hosang | ||
| William Haddock | Bill Roach | Alexander Landmann | ||
| Svetlana Khodchenkova | Irina | Morin Smolé | ||
| Kathy Burke | Connie Sachs | Marie Gruber | ||
| Imre Csuja | KGB-Agent | Victor Choulman | ||
| Christian McKay Christian McKay | Mackelvor | F.G.M. Stegers | ||
| Roger Lloyd Pack | Mendel | Peter Reinhardt Peter Reinhardt | ||
| Konstantin Khabenskiy | Polyakov | Waléra Kanischtscheff | ||
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