| Schauspieler | Rolle | Synchronsprecher | ||
| Nicole Kidman Nicole Kidman | Marisa Coulter | Petra Barthel Petra Barthel | ||
| Daniel Craig Daniel Craig | Lord Asriel | Dietmar Wunder Dietmar Wunder | ||
| Dakota Blue Richards | Lyra Belacqua | Lisa May-Mitsching | ||
| Charlie Rowe | Billy Costa | David Wittmann | ||
| Paul Antony-Barber | Bolvangar Doctor | Bernd Vollbrecht Bernd Vollbrecht | ||
| Jason Watkins | Bolvangar Official | Hans Hohlbein Hans Hohlbein | ||
| Simon McBurney | Fra Pavel | Oliver Rohrbeck Oliver Rohrbeck | ||
| Tom Courtenay | Farder Coram | Friedhelm Ptok | ||
| Sir Christopher Lee Sir Christopher Lee | Hoher Rat des Magisteriums | Otto Mellies | ||
| Joao de Sousa | Hunt | Jaron Löwenberg Jaron Löwenberg | ||
| John Franklyn-Robbins | Librarian | Jochen Schröder Jochen Schröder | ||
| Sam Elliott Sam Elliott | Lee Scoresby | Jürgen Kluckert Jürgen Kluckert | ||
| Jim Carter | Lord John Faa | Engelbert von Nordhausen Engelbert von Nordhausen | ||
| Clare Higgins | Ma Costa | Heidrun Bartholomäus Heidrun Bartholomäus | ||
| Sir Derek Jacobi | Magisterial Emissary | Lutz Mackensy Lutz Mackensy | ||
| Jack Shepherd | Master | Friedrich Georg Beckhaus Friedrich Georg Beckhaus | ||
| Ben Walker | Roger | Leo Vornberger | ||
| Magda Szubanski | Mrs. Lonsdale | Marianne Groß Marianne Groß | ||
| Hattie Morahan | Schwester Clara | Ulrike Stürzbecher Ulrike Stürzbecher | ||
| Eva Green Eva Green | Serafina Pekkala | Tanja Geke Tanja Geke | ||
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